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Metal-Free Hydrogenation of Imines Catalyzed by B(C6F5)3

Stephan et al. have reported the metal-free hydrogenation of imines catalyzed by B(C6F5)3. According to their results, catalytic transfer hydrogenation of imines, enamines, and N-heterocycles is demonstrated by exploiting the activation of amines by the Lewis acid B(C6F5)3. This method has attracted much attention because it represents a rare example of metal-free transfer hydrogenation and can employ the readily accessible diisopropylamine as the source of hydrogen.

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